Manufacturing Technology 2021, 21(3):330-339 | DOI: 10.21062/mft.2021.036

Development and Evaluation of a Thin Cerium Oxide-Gelatin Nanolaminate Coating for Corrosion Protection of AISI 316L Stainless Steel

Mohammed T. Hayajneh ORCID..., Mohammed Almomani ORCID..., Mohammad Al-Daraghmeh ORCID...
Industrial Engineering Department, Faculty of Engineering, Jordan University of Science and Technology P.O. Box 3030, Irbid, 22110, Jordan

AISI 316L stainless steel is widely used for multiple applications because of its good mechanical properties and corrosion resistance in multiple environments. However, the long exposure of AISI 316L steel to aggressive environments containing chloride ions limits its electrochemical performance significantly. The objective of this research is to develop and evaluate a thin cerium oxide-gelatin nanolaminate coatings for corrosion protection of the spin-coated AISI 316L stainless steel in 3.5% NaCl solution as the corrosion medium. The nanolaminate coat-ings were evaluated by the potentiodynamic polarization technique and the characterization of the coatings was performed by using XRD, SEM, and EDX. The results show that the corrosion behaviour of CeO2-gelatin nano-laminate coatings significantly improves the corrosion behaviour of the coated AISI 316L steel. The results also confirm the formation of homogeneous and crack-free coatings without any noticeable defect. One-way ANOVA analysis was used to examine the statistical significance of coating types. The novelty of this research is the development and preparing nanocomposites coatings by using gelatin as a gel matrix for nanocomposites powder dis-persion instead of the traditional methods to improves the uniform and localized corrosion of the AISI 316L steel. The results showed that the prepared coatings significantly improved the uniform and localized corrosion resistance of the AISI 316L steel.

Keywords: Corrosion evaluation, Nanolaminate coating, Cerium oxide, Gelatin, AISI 316L stainless steel, Spin coating.
Grants and funding:

Supported by a grant from the Deanship of Scientific Research at Jordan University of Science and Technology (JUST) with grant no. 39/2017.

Received: July 19, 2020; Revised: March 24, 2021; Accepted: April 7, 2021; Prepublished online: April 8, 2021; Published: June 7, 2021  Show citation

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Hayajneh MT, Almomani M, Al-Daraghmeh M. Development and Evaluation of a Thin Cerium Oxide-Gelatin Nanolaminate Coating for Corrosion Protection of AISI 316L Stainless Steel. Manufacturing Technology. 2021;21(3):330-339. doi: 10.21062/mft.2021.036.
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References

  1. ASHRAFI, A., GOLOZAR, M., MALLAKPOUR, S. (2009). Corrosion behaviour of 316L stainless steel coated by amorphous and semicrystalline polypyrrole. Surface Engineering, Vol. 25, No. 2, pp. 120-126. Go to original source...
  2. ZHAO, Y., ZHOU, F., YAO, J., DONG, S., LI, N. (2015). Erosion-Corrosion Behaviour and corrosion resistance of AISI 316 stainless steel in flow jet impingement. Wear, Vol. 328-329, pp. 464-476. Go to original source...
  3. MAJEDI, A., DAVAR, F., ABBASI, A., ASHRAFI, A. (2016). Modified sol-gel based nanostructured zirconia thin film: preparation, characterization, photocatalyst and corrosion behavior. Journal of Inorganic and Organometallic Polymers and Materials, Vol. 26, No. 5, pp. 932-942. Go to original source...
  4. BOTTOLI, F., JELLESEN, M., CHRISTIANSEN, T., WINTHER, G., SOMERS, M. (2018). High temperature solution-nitriding and low-temperature nitriding of AISI 316: effect on pitting potential and crev-ice corrosion performance. Applied Surface Science, Vol. 431, pp. 24-31. Go to original source...
  5. ALMOMANI, M., AITA, C. (2009). Pitting Corrosion Protection of Stainless Steel by Sputter Deposited Haf-nia, Alumina, and Hafnia-Alumina Nanolaminate Films. Journal of Vacuum Science & Technology A, Vol. 27, No. 3, pp. 449. Go to original source...
  6. RICCARDO, BALZAROTTI, CINZIA CRISTIANI, SAVERIO LATORRATA, ALESSANDRO MIGLIAVACCA. (2015). Washcoating of low surface area cerium oxide on complex geometry sub-strates. Particulate Science and Technology, Vol. 34, No. 2, pp. 184-193. Go to original source...
  7. DRÁPALA, J., MACHOVČÁK, P., JONŠTA, P., HA, VT., BROŽOVÁ, S., KOSTIUKOVÁ, G., MADAJ, M. (2015). Structural Characteristics of Cr-Mo Steels Microalloyed with Cerium. Manufacturing Technology, Vol. 15, No. 3, pp. 315-322. Go to original source...
  8. ARORA, S., MESTRY, S., SINGH H, K., MHASKE, S. (2020). Sol-gel based layer-by-layer deposits of lanthanum cerium molybdate nanocontainers and their anticorrosive attributes. Iranian Polymer Journal, Vol. 29, pp. 133-146. Go to original source...
  9. DANAEE, I., DARMIANI, E., RASHED, G. R., ZAAREI, D. (2014). Self-healing and anticorrosive properties of Ce(III)/Ce(IV) in nanoclay-epoxy coatings. Iranian Polymer Journal, Vol. 23, pp. 891-898. Go to original source...
  10. SHI, Z., ZHOU, Z., SHUM, P., LI, L. (2019). Thermal stability, wettability and corrosion resistance of sputtered ceria films on 316 stainless steel. Applied Surface Science, Vol. 477, pp. 166-171. Go to original source...
  11. XU, J., XIN, S., HAN, P., MA, R., LI, M. (2013). Cerium chemical conversion coatings for corrosion protection of stainless steels in hot seawater environments. Material and Corrosion, Vo. 64, No. 7, pp. 619-624. Go to original source...
  12. HAYAJNEH, MT., ALMOMANI, M., AL-DARAGHMEH, M. (2019). Enhancement the Corrosion Resistance of AISI 304 Stainless Steel by Nanocomposite Gelatin-Titanium Dioxide Coatings. Manufacturing Technology, Vol. 19, No. 5, pp. 759-766. Go to original source...
  13. ZHONG, S., ZHANG, Y., LIM, C. (2010). Tissue scaffolds for skin wound healing and dermal reconstruction. Wiley Interdisciplinary Reviews Nanomedicine and Nanobiotechnology, Vo. 2, No. 5, pp. 210-525. Go to original source...
  14. DILLE, M., HATTREM, M., DRAGET, K. (2018). Soft, chewable gelatin-based pharmaceutical oral formulations: a technical approach. Pharmaceutical Development and Technology, Vol. 23, No. 5, pp. 504-511. Go to original source...
  15. AL-DARAGHMEH, M., ALMOMANI, M., HAYAJNEH, M. (2019). Corrosion Resistance of TiO2-ZrO2 Nanocomposite Thin Films Spin Coated on AISI 304 Stainless Steel in 3.5 wt. % NaCl Solution. Materials Research, Vol. 22, No. (5), pp. 1-9. Go to original source...
  16. ALMOMANI, M., HAYAJNEH, M., AL-DARAGHMEH, M. (2019). The corrosion behavior of AISI 304 stain-less steel spin coated with ZrO2 -gelatin nanocomposites. Mater Res Express, Vol. 6, No. 9, pp. 65c4. Go to original source...
  17. HAYAJNEH, M., ALMOMANI, M., AL_HMOUD, H. (2019). Corrosion evaluation of nanocomposite gelatin-forsterite coating applied on AISI 316L stainless steel. Mater Res Express, Vol. 6, No. 11, pp. 6431. Go to original source...
  18. SVOBODOVA, J., LUNAK, M., LATTNER, M. (2019). Analysis of the Increased Iron Content on the Corrosion Resistance of the AlSi7Mg0.3 Alloy Casting. Manufacturing Technology. Vol. 19, No. 6, pp. 1041-1046. Go to original source...
  19. ESWARA KRISHNA, M., PATOWARI P, K. (2013). Parametric optimisation of electric discharge coating process with powder metallurgy tools using Taguchi analysis. Surface Engineering, Vol. 29, No. 9, pp. 183-189. Go to original source...
  20. ALMOMANI, M., HAYAJNEH, M., ALELAUMI, S. (2019). Applying Taguchi method to study the wear behaviour of ZA-27 alloy-based composites reinforced with SiC nanoparticles. International Journal of Cast Metals Research, Vol. 32, No. 4, pp. 229-241. Go to original source...
  21. PAL, K., BANTHIA, AK., MAJUMDAR, DK. (2007). Preparation and characterization of polyvinyl alcohol-gelatin hydrogel membranes for biomedical applications. AAPS PharmSciTech, Vol. 8, No. 1, pp. E142-E146. Go to original source...
  22. TORKAMAN, R., DARVISHI, S., JOKAR, M., KHARAZIHETA, M., KARBASI, M. (2017). Electro-chemical and in Vitro Bioactivity of Nanolaminate Gelatin-Forsterite Coatings on AISI 316 L Stainless Steel. Progress in Organic Coatings, Vol. 103, pp. 40-47. Go to original source...

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